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By Herbert D. Kaesz

Content material: bankruptcy 1: Main-group compounds -- normal -- bankruptcy 2: Boron compounds -- bankruptcy three: Transition steel coordination compounds -- bankruptcy four: Transition steel organometallics and ligands -- bankruptcy five: Cluster and cage compounds containing transition metals

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60. 61. 62. 63. 64. 65. 66. 67. 68. 69. , J. Am. Chem. Soc. 1984, 106, 5145–5150. , Cytochromes c: Evolutionary, Structural, and Physicochemical Aspects. Springer-Verlag: New York, 1990; p. 478. , Cytochrome c - A Multidisciplinary Approach. University Science Books: Sausalito, CA, 1996; p. 738. , J. Am. Chem. Soc. 1988, 110, 429–434. , J. Am. Chem. Soc. 1979, 101, 883–892. , J. Am. Chem. Soc. 1991, 113, 7056–7057. , Proc. Natl. Acad. Sci. USA 1991, 88, 1325–1329. , Isr. J. Chem. 1981, 21, 8–12.

The occupancy of narrow cavities with water molecules is a sensitive function that is strongly dependent on the strength of the interactions with the cavity wall. Thus even subtle changes in these interactions can cause transitions between an empty and a full cavity22. Such behaviour may well explain why the cavity in cytochrome c oxidase appears empty by X-ray crystallographic criteria, but appears to be filled at least transiently with 3–4 water molecules during dynamic turnover. Kornblatt23 has shown in elegant experiments that the electron transfer from haem a to the binuclear site in cytochrome c oxidase depends on the presence of water molecules within the protein.

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